First thing that could simplify your code is the fact that the string is an array of chars. For example try what happens with the following code
string str = "aabb12cc";
Console.WriteLine(str[3]);
Having that said, you could have a single loop looping through all the characters and if the character is desired one, then increment the counter by one. A simple loop could be a
for (C# Reference)[
^] loop starting from 0 and ending at the end of the string.