I think you are very close to being able to make this work: just focus on the fact that the moment one of the +-*/ operator buttons is pressed you need:
1. to store the value in the TextBox,
as well as which operator was pressed
2. when the = operator button is pressed you need to get the second value, and then execute the stored operator, using the first value entered
I suggest you make the = operator button Click EventHandler a separate function in order to do this. I also suggest you switch to using 'double, not Int32, since you will lose all fractional values using Int32.
Here's a rough outline in psuedo-code:
private double firstValue;
private string operatorToExecute;
private void ActionOperator_Click((object sender, EventArgs e))
{
operatorToExecute =
firstValue =
}
private void EqualOperator_Click()
{
double secondValue =
}